Microwave-optical spectroscopy of Rydberg excitons in the ultrastrong driving regime

Abstract

We study the ultrastrong driving of Rydberg excitons in Cu _2 O by a microwave field. The effect of the field is studied using optical absorption spectroscopy, and through the observation of sidebands on the transmitted laser light. A model based on Floquet theory is constructed to study the system beyond the rotating wave approximation. We obtain near quantitative agreement between theory and experiment across a 16-fold range of microwave field strengths spanning from the perturbative to the deep strong driving regime. Compared to Rydberg atoms, the large non-radiative widths of Rydberg excitons leads to new behaviour such as the emergence of an absorption continuum without ionization.

Keywords

• Rydberg excitons
• strong driving
• ultrastrong driving
• ultrastrong coupling
• Floquet theory
• microwave optical conversion